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Defective silicalite-1 is an efficient and selective catalyst in gas phase Beckmann rearrangement. A kinetic study of catalyst decay applied to Beckmann reaction of cyclohexanone oxime into ɛ-caprolactam performed with silicalite-1 as catalyst was carried out with reference to time on stream theory. Information about kinetic deactivation constant was obtained. Kinetic deactivation expressions based...
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