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The quantum yield for light-induced H2 generation was measured for a previously optimized bio-hybrid cytochrome c6-crosslinked PSIC13G–1,8-octanedithiol–[FeFe]-H2aseC97G (PSI–H2ase) nanoconstruct. The theoretical quantum yield for the PSI–H2ase nanoconstruct is 0.50 molecules of H2 per photon absorbed, which equates to a requirement of two photons per H2 generated. Illumination of the PSI–H2ase nanoconstruct...
Two‐dimensional photosynthetic protein crystals provide a high density of aligned reaction centers. We reconstitute the robust light harvesting protein Photosystem I into a 2D crystal with lipids and integrate the crystals into a photo‐electrochemical device. A 4‐fold photocurrent enhancement is measured by incorporating conjugated oligoelectrolytes to form a supporting conductive bilayer in the device...
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