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To search for alternative electrostrictive polymers and to understand the underlying mechanism, the structure‐ferroelectric/electrostrictive property relationship for nylon‐12‐based poly(ether‐b‐amide) multiblock copolymers (PEBAX) is investigated. Two PEBAX samples are studied, namely, P6333 and P7033 with 37 and 25 mol.% of soft poly(tetramethylene oxide) (PTMO) blocks, respectively. In both samples,...