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Reduction methods for the preparation of coordination complexes of titanium(IV) and indium(III) phthalocyanines (Pc) with organic dyes such as indigo, thioindigo, and squarylium dye III (SQ) have been developed, which allow one to obtain crystalline {cryptand(K+)}{(cis‐indigo‐O,O)2−TiIV(Pc2−)}(Cl−)⋅C6H4Cl2 (1), {cryptand(K+)}{(cis‐thioindigo‐O,O)2−InIII(Pc2−)}−⋅C6H4Cl2 (2), and {cryptand(K+)}{[(SQ)...