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Engineering self‐templating inorganic architectures is critical for the development of bottom‐up approaches to nanoscience, but systems with a hierarchy of templates are elusive. Herein we describe that the cluster‐anion‐templated (CAT) assembly of a {CAT}⊂{Mo24Fe12} macrocycle forms a giant ca. 220 nm3 unit cell containing 16 macrocycles clustered into eight face‐shared tetrahedral cluster‐of‐clusters...
Eine Reihe von Supermolekülen, …… die als Eigentemplate fungieren, öffnet den Zugang zu einem neuen Universum anorganischer Makrocyclen, wie L. Cronin et al. in der Zuschrift auf S. 12895 ff. beschreiben. Im Bild sind die {Mo24Fe12}‐Makrocyclen zu sehen, die in dem durch den zentralen Hohlraum gebildeten makrocyclischen Raum Keggin‐, Dawson‐, Anderson‐ und hexalakunäre Polyoxometallatcluster vom Dawson‐Typ...
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