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Proteins of thermophiles are thermally stable in a high‐temperature environment, adopting a strategy of enhancing the electrostatic interaction in hydrophobic media at high temperature. Herein, inspired by the molecular mechanism of thermally stable proteins, the synthesis of novel polymer materials that undergo ultrarapid, isochoric, and reversible switching from soft hydrogels to rigid plastics...
Polymeric hydrogels showing ultrafast modulus jump of 1800‐folds by heating is achieved by Takayuki Nonoyama, Jian Ping Gong, and co‐workers in article number 1905878. Like proteins in thermophiles, the hydrogels robustly dehydrate by heating due to interplay of hydrophobic and ionic interactions. The strong microscale phase separation induces vitrification to show rubbery–glassy transition by heating...
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