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Calculated CO stretching frequencies for the Rh(111)-(2x2)-3CO structure are compared with recent high-resolution electron energy loss spectroscopy (HREELS) experiments. Two loss peaks in the HREELS spectrum at 2070 and 1861 cm -1 were attributed to ontop- and hollow-bonded CO molecules, respectively. Two weaker peaks, which had not been observed before due to the lack of resolution,...
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