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The preparation of homo‐ and heterocomplexes composed of the parent perylene diimide (PH) and pyrrolidine‐substituted perylene diimide (PN) in DNA and rapid electron transfer in these complexes, which has been analyzed by steady‐state fluorescence and femtosecond transient absorption measurements, have been demonstrated. The DNA molecules possessing PH and PN were prepared through a recently developed...
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