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Anode‐free solid‐state batteries (AFSSBs) are considered to be one of the most promising high‐safety and high‐energy storage systems. However, low Coulombic efficiency stemming from severe deterioration on solid electrolyte/current collector (Cu foil) interface and undesirable Li dendrite growth impede their practical application, especially when rigid garnet electrolyte is used. Here, an interfacial...
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