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Chained melody: Ubiquitination is forged through the nonstandard isopeptide bond between the ε‐nitrogen atom of a lysine residue on a target protein and the C‐terminal carboxy group of ubiquitin. Several complementary synthetic approaches have led to designated diubiquitin chains in quantities useful for structure–function analyses, culminating in the total chemical synthesis of all seven diubiquitin...
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