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Solid polymer electrolytes with large ionic conductivity, high ionic transference number, and good interfacial compatibility with electrodes are highly desired for solid‐state batteries. However, unwanted polarizations and side reactions occurring in traditional dual‐ion polymer conductors hinder their practical applications. Here, single‐ion polymer conductors (SIPCs) with exceptional selectivity...
Polymer‐based electrolytes have attracted ever‐increasing attention for all‐solid‐state lithium (Li) metal batteries due to their ionic conductivity, flexibility, and easy assembling into batteries, and are expected to overcome safety issues by replacing flammable liquid electrolytes. However, it is still a critical challenge to effectively block Li dendrite growth and improve the long‐term cycling...
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