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The relatively low resistivity and severe ion migration in CsPbBr3 significantly degrade the performance of X‐ray detectors due to their high detection limit and current drift. The electrical properties and X‐ray detection performances of CsPbBr3−nIn single crystals are investigated by doping the iodine atoms into the melt‐grown CsPbBr3. The resistivity of CsPbBr3−nIn single crystals increases from...