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We theoretically analyzed the glucose oxidation reaction mechanism and reaction activity of Au catalyst supported by carbon (graphite(0001), (1 0 1¯ 0), and (1 1 2¯ 0)) and oxide (ZrO2(111) and SnO2(110)) in alkaline solution environment by using density functional theory method. We observed large stabilization of Au catalyst on support materials due to the electron transfer in the case of graphite(1...
We theoretically analyzed the surface structure of Au in alkaline solution and the glucose oxidation reaction to understand the electrooxidation process in direct alkaline glucose fuel cell. We find the oxidation reaction mechanism of glucose on Au catalyst in alkaline solution theoretically as follows. i) Glucose adsorbs on OH of Au surface. ii) OH− in alkaline solution interacts with CHO group of...
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