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Two-photon ionization of the nickelocene molecules cooled in a supersonic jet was performed for the first time by simultaneous excitation of (η5−C5H5)2Ni with two tunable nano- second dye lasers. The one-photon transition from the HOMO to the Rydberg R4p level was used as the initial step of the multiphoton excitation. In a one-color experiment, the conditions were found for generation of the intact...
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