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Here a method is presented for the temperature‐switchable assembly of viral particles into large hierarchical complexes. Dual‐functional diblock copolymers consisting of poly(diethyleneglycol methyl ether methacrylate) (poly(DEGMA)) and poly((2‐dimethylamino)ethyl methacrylate) (poly(DMAEMA)) blocks self‐assemble electrostatically with cowpea chlorotic mottle virus (CCMV) particles into micrometer‐sized...
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