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Temperature dependent Raman spectra of the crystals CsCdCl3 and CsCdBr3 grown by Bridgman method were measured in the temperature range of 5–300K.The description of the line-broadening and the line-shift of the observed Raman lines are mainly based on the anharmonicity due to the phonon–phonon interaction. The analysis of the temperature dependence of the Raman-lines that involve vibrational modes...
The excitation and emission spectra of CsCdCl 3 crystal grown by the Bridgman growth technique, are observed. Its dominant excitation spectra correspond to the transitions between the electronic energy levels of the face-shared [CdCl 6 ] 4− octahedron complexes with C 3v symmetry. With the help of the molecular orbital diagram of the [CdCl 6 ] 4− molecule...
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