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The syntheses, structures, and chemotherapeutic activities of Ag(I)‐, Au(I)‐, and Ru(II)‐complexes ligated to a novel N‐heterocyclic carbene ligand, 2‐(4‐nitrophenyl)imidazo[1,5‐a]pyridin‐2‐ylidene (1), are described. The corresponding complexes, [Ag(1)2][PF6], [Au(1)2][PF6] (3), and [Ru(1)(p‐cymene)Cl][PF6] (4), were prepared using convenient transmetallation chemistry and characterized using a range...