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Molecular‐level insight into interfacial water at a buried electrode interface is essential in electrochemistry, but spectroscopic probing of the interface remains challenging. Here, using surface‐specific heterodyne‐detected sum‐frequency generation (HD‐SFG) spectroscopy, we directly access the interfacial water in contact with the graphene electrode supported on calcium fluoride (CaF2). We find...
Molekulare Einblicke in Wasser an Elektrodengrenzflächen sind für die Aufklärung vieler elektrochemischer Phänomene, unter Anderem der elektrokatalytischen Wasserspaltung und der kapazitiven Energiespeicherung, von wesentlicher Bedeutung, aber die spektroskopische Untersuchung dieser Grenzflächen bleibt eine Herausforderung. Mit Hilfe der oberflächenspezifischen heterodyn‐detektierten Summenfrequenzspektroskopie...
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