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The isoreticular metal–organic framework (MOF) UiO‐66‐X with diverse functional groups, encapsulating guest Pd nanoparticles, is fabricated by H.‐L. Jiang and co‐workers, as described in article number 2000041. The chemical microenvironment around the Pd is systematically regulated by these MOF hosts, giving rise to distinctly different performances toward the hydrogenation of benzoic acid.
The chemical environment of metal nanoparticles (NPs) possesses significant influence on their catalytic performance yet is far from being well understood. Herein, tiny Pd NPs are encapsulated into the pore space of metal–organic frameworks (MOFs), UiO‐66‐X (X = H, OMe, NH2, 2OH, 2OH(Hf)), affording Pd@UiO‐66‐X composites. The surface microenvironment of the Pd NPs is readily modulated by pore wall...
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