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In article number 1703151, Ling‐Hai Xie, Li‐Tao Sun, Wei Huang, and co‐workers propose a general strategy for programmable 2D organic nanosheets formation based on the synergistically molecular attractor‐repulsor theory (SMART). As a typical attractor‐repulsor model molecule, TPA‐PF is made up of a supramolecular segment TPA and a bulky group PF. The synergetic effect between them leads to an interdigital...
Rational molecular design for the organic nanocrystal morphology still remains a challenge due to the structural diversity and complicated weak intermolecular interactions. In this work, a typical attractor–repulsor molecule N,N‐diphenyl‐4‐(9‐phenyl‐fluoren‐9‐yl) phenylamine (TPA‐PF) is designed to explore a general assembly strategy for 2D nanocrystals. Via an interdigital lipid bilayer‐like (ILB)...
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