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2D 2H‐phase MoS2 is promising for electrocatalytic applications because of its stable phase, rich edge sites, and large surface area. However, the pristine low‐conductive 2H‐MoS2 suffers from limited electron transfer and surface activity, which become worse after their highly likely aggregation/stacking and self‐curling during applications. In this work, these issues are overcome by conformally attaching...