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The fracture toughness of two alkoxysilane modified bis‐phenol‐A (BPA) epoxides were compared at three different temperatures. Organosilanes were utilized to synthesize the modified epoxides; 3‐aminopropyl triethoxysilane reacted with the telechelic oxirane (aminosilane functionalized epoxide, ASE); and 3‐(triethoxysilyl) propyl isocyanate reacted with the secondary hydroxyl group of the repeat unit...