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The preparation and electronic properties of Cs1−xAxAl0.33Te1.67O6 (A = K, Rb, and Cs) are reported. Replacing Cs with smaller Rb and K reduces cell parameters of the compounds but does not affect the overall structure. Electronic conductivities of all samples were measured and explained based on the band conduction model. Although XPS Te3d5/2 spectra indicate that all samples contain similar amount...