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We present an optimization course analysis of two coherent control experiments optimizing the ion yield in NaK and the isotope ratio of 39,39 K 2 / 39,41 K 2 with shaped laser pulses. As most evolutionary algorithms converge first to the most relevant parameters qualitative information about their importance can be extracted. Additional information is gained by comparing...
Frequency dependent closed loop optimization of fs pulse shapes is investigated for the NaK dimer. By controlling the photo-excited wave packet dynamics, the three-photon ionization of NaK is optimized. The obtained ion yield depending on the employed central laser frequency shows a maximum in the range of 770-780 nm. By investigating the modifications of the optimal pulse shapes for different wavelengths...
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