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A new gas-phase infrared (IR) spectrum of acryloyl fluoride (ACRF, CH2CHCFO) with a resolution of 0.1cm−1 in the range 4000–450cm−1 was measured. Theoretical ab initio molecular structures, full quartic potential energy surfaces (PES), and cubic surfaces of dipole moments and polarizability tensor components (electro-optical properties, EOP) of the s-trans and s-cis conformers of the ACRF were calculated...
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