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A microkinetic model is developed for the NO-oxidation on platinum. The approach we followed employs semi-empirical methods, optimization of the parameters of elementary-like reactions, and thermodynamic constraints. The model is capable of capturing reasonably light-off experimental data.
The influence of reaction exothermicity and transport of species on the bifurcation behavior of CH 4 /air mixtures is studied in a continuous stirred tank reactor with numerical bifurcation techniques, using the 177-reaction/31-species Gas Research Institute mechanism, version 1.2. Ignition points are analyzed through various sensitivity analyses, quasi-steady-state analysis, and numerical...
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