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A squaraine dye is tested for novel application in a near‐infrared‐active organic photovoltaic cell that is subsequently optimized to obtain a power conversion efficiency of 2.4 ± 0.3%. The optimization utilizes an Alq3 buffer layer and macroscopic structure control through the addition of co‐solvents in the spin‐casting process. Co‐solvent addition increases the amount of aggregates present as measured...
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