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Free‐standing polypeptide films are formed by a novel cross‐linking pathway involving cross‐chain terminations of polypeptide chains grown from multifunctional initiators. Greg G. Qiao, Frank Caruso, and co‐workers describe on page 4619 how this fabrication method provides a facile approach towards the formation of stable cross‐linked polypeptide capsules with tunable thickness, compositions, and...
Cross‐linked polypeptide‐based films are fabricated via a novel and robust method employing surface‐initiated ring opening polymerization of α‐amino acid N‐carboxyanhydrides (NCA‐ROP). The judicious combination of amine‐based hyperbranched macroinitiators and benzyl ester‐protected NCA derivatives promotes network formation by cross‐chain terminations, which allows the formation of stable cross‐linked...
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