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The issue of localization/delocalization of electron spin density in Metal-to-Ligand Charge Transfer (MLCT) excited states of [Ru(bpy)3]2+ (bpy=2,2′-bipyridine) has been debated for almost four decades. Localization/delocalization of MLCT excited states specifically addresses the question regarding electron configuration in the excited state and whether the excited electron in the dπ5π∗1 excited state...
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