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The correlation of the remarkable solvatochromism and solvent-dependent deuteron NMR spectra of fac-[CrF 3 (tpa)] (tpa=tri(2-pyridyl)amine) with the acceptor numbers (A N s) for solvents demonstrated the sensitivity of the Cr ligand bond length or the angular overlap model (AOM) parameters to the embedding solvent, and also suggested a significant trigonal splitting in the first ...