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Constructing dynamic covalent bonds (DCBs) in rubbers provides a promising avenue to resolve the trade‐offs between chemical crosslinking and recyclability. The reinforcement of dynamic covalent networks by nanofilling is widely adopted, which, however, inevitably hinders the exchange reaction of DCBs and network rearrangement due to the restrictions on chain mobility imposed by fillers. To date,...
Upcycling of cross‐linked rubbers is pressing. The introduction of dynamic covalent bonds into the networks is a popular tactic for recycling thermosetting polymers, but it is very challenging to integrate engineering performance and continuous yet stable reprocessability. Based on traditional rubber formulations, herein, a straightforward strategy is presented for constructing a skeletal network...