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Ta3N5 is a promising photoanode candidate for photoelectrochemical water splitting, with a band gap of about 2.1 eV and a theoretical solar‐to‐hydrogen efficiency as high as 15.9 % under AM 1.5 G 100 mW cm−2 irradiation. However, the presently achieved highest photocurrent (ca. 7.5 mA cm−2) on Ta3N5 photoelectrodes under AM 1.5 G 100 mW cm−2 is far from the theoretical maximum (ca. 12.9 mA cm−2),...
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