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Water electrolysis is an ideal method for industrial green hydrogen production. However, due to increasing scarcity of freshwater, it is inevitable to develop advanced catalysts for electrolyzing seawater especially at large current density. This work reports a unique Ru nanocrystal coupled amorphous‐crystal Ni(Fe)P2 nanosheet bifunctional catalyst (Ru‐Ni(Fe)P2/NF), caused by partial substitution...