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The synthesis, spectral and magnetic characterization and the molecular and 3D structure of a double dicyanamide-bridged Cu(II) chain compound are described. The axial ligands are 4-Mepyrimidine. The Jahn–Teller axis of the Cu(II) ion is directed towards one dicyanamide pair (Cu-N=2.393Å); the short Cu-N distances are around 2.00Å. Magnetic exchange interactions between the Cu(II) ions are weak, as...
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