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The synthesis, variable-temperature electronic absorption spectroscopy, magnetic susceptibility of a novel valence tautomer are presented, and thermodynamic parameters for the valence tautomeric equilibrium were determined. The dioxolene used is a semiquinone–nitronylnitroxide donor–acceptor ligand. Due to the ferromagnetic coupling inherent in the semiquinone–nitronylnitroxide donor–acceptor biradical,...
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