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The accurate study of the electron transfer activity of the tetraanion [Pt19(CO)22]4− is presented together with that of the dianion [Pt38(CO)44]2−, which was previously studied by spectroelectrochemistry but only partially examined from the electrochemical viewpoint. The main feature of the two clusters is that they undergo a sequence of close-spaced pairs of reversible one-electron processes, which...
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