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A dimanganese tetrakis-Schiff base complex [MnII2L]2+, where L provides a N6O2 coordination environment, has been synthesized and characterized via electrochemical and spectroscopic studies. Cyclic voltammograms (CV) of [MnII2L]2+ in propylene carbonate, to which water has been added as a limiting reagent, show an increase in current starting at +1.3V versus Fc+/0. The current shows a first order...
Intervalence Stark effect spectroscopy of a symmetrically substituted and an asymmetrically substituted derivative of the Creutz–Taube ion, (NH3)5Ru-pyrazine-Ru(NH3)55+, is reported. Like the formally mixed-valent parent ion, both appear to lie near the boundary between valence delocalization and valence localization. Remarkably, despite the close structural similarities of the two compounds investigated,...
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