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Architecture-regulated cellulose derivatives were prepared by regioselective substitution of C-2, -3, and -6 position hydroxyls in cellulose by O-acetyls or trityls. Their dynamic structures formed in polar solvents were compared with those by the commercial cellulose acetates where the distribution of hydroxyls and O-acetyls was nearly random in the chain. It was found that the difference in the...
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