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By combining metal‐organic frameworks (MOFs) with colloidal crystals, the challenge of signal transduction in response to molecular sorption by MOF materials can be met for sensing applications. HKUST‐1 (Cu2(BTC)3) is grown on a silica colloidal crystal thin film via a step‐by‐step technique, and the obtained MOF‐containing colloidal crystal is rapidly and reversibly responsive to vapor or gas molecules...
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